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Collective electromagnetic emission from molecular layers on metal nanostructures mediated by surface plasmons

Collective electromagnetic processes stemming from molecular emission close to complex nanostructured metal surfaces pumped at and/or near surface-plasmon resonances are theoretically investigated. A classical electrodynamics model is used to describe macroscopically the surface molecular layer emission. Generalized Fresnel coefficients are analytically obtained for planar surfaces, indeed predicting collective quenching for redshifted emission at given angles. The model is introduced into a ...

Electromagnetic model and calculations of the surface-enhanced Raman-shifted emission from Langmuir-Blodgett films on metal nanostructures

We present a theoretical study of the electromagnetic contribution to surface-enhanced Raman scattering (SERS) from a Langmuir-Blodgett film close to a metal surface. This macroscopic dipolar model fully accounts for the Raman-shifted emission so that meaningful SERS (electromagnetic) enhancement factors that do not depend only on the local electromagnetic field enhancement at the pump frequency are defined. For a plane metal surface, analytical SERS enhancement factors that are consistent fo...