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Oxford University Research Archive
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13393 Publications
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  • Moving & feeling

    This thesis focuses on tactile perception and aims at a comprehensive analysis of its characteristics over the time-course of various goal-directed movements. Tactile perception is assessed by means of discrimination and detection paradigms, as well as event-related potentials (ERPs). The main question investigated throughout the thesis is: ‘What changes in tactile perception, if any, take place over the time course of a goal-directed movement?’ In Chapter 2, the mechanisms related to such id...

    DifFUZZY: a novel clustering algorithm for systems biology

    Ornella Cominetti Allende (2012)
    Current studies of the highly complex pathobiology and molecular signatures of human disease require the analysis of large sets of high-throughput data, from clinical to genetic expression experiments, containing a wide range of information types. A number of computational techniques are used to analyse such high-dimensional bioinformatics data.In this thesis we focus on the development of a novel soft clustering technique, DifFUZZY, a fuzzy clustering algorithm applicable to a larger class o...

    The impact of stochastic physics on tropical rainfall variability in global climate models on daily to weekly time scales

    Watson, P; Berner, J; Corti, S; Davini, P; von Hardenberg, J; Sanchez, C; Weisheimer, A; Palmer, TN (2017)
    Many global atmospheric models have too little precipitation variability in the tropics on daily to weekly time scales, and also poor representation of tropical precipitation extremes associated with intense convection. Stochastic parameterisations have the potential to mitigate this problem by representing unpredictable subgrid variability that is left out of deterministic models. We evaluate the impact on the statistics of tropical rainfall of two stochastic schemes, the stochastically pe...

    Formation of a σ-alkane Complex and a Molecular Rearrangement in the Solid-State: [Rh(Cyp2PCH2CH2PCyp2)(η2:η2-C7H12)][BArF4]

    McKay, AI; Krämer, T; Rees, NH; Thompson, AL; Christensen, KE; Macgregor, SA; Weller, Andrew (2016)
    Addition of H2 to the precursor [Rh(Cyp2P(CH2)2PCyp2)(η2 :η2 -C7H8)][BArF 4] gives the σ-alkane complex [Rh(Cyp2P(CH2)2PCyp2)(η2 :η2 -C7H12)][BArF 4] by a single-crystal to single–crystal reaction, as characterized by X-ray crystallography, SSNMR spectroscopy and periodic DFT. An unexpected rearrangement of the {Rh(L2)}+ fragment is revealed.

    New titanium borylimido compounds: synthesis, structure and bonding

    Clough, BA; Mellino, S; Protchenko, AV; Slusarczyk, M; Stevenson, LC; Blake, MP; Xie, B; Clot, E; Mountford, P (2017)
    We report a combined experimental and computational study of the synthesis and electronic structure of titanium borylimido compounds. Three new synthetic routes to this hitherto almost unknown class of Group 4 imide are presented. The double-deprotonation reaction of the borylamine H2NB(NAr'CH)2 (Ar' = 2,6-C6H3 i Pr2) with Ti(NMe2)2Cl2 gave Ti{NB(NAr'CH)2}Cl2(NHMe2)2 which was easily converted to Ti{NB(NAr'CH)2}Cl2(py)3. This compound is an entry point to other borylimide...
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