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Han, Guang; Popuri, Srinivas R.; Greer, Heather F.; Ferre Llin, Lourdes; Bos, Jan-Willem G.; Zhou, Wuzong; Paul, Douglas J.; Ménard, Hervé; Knox, Andrew R.; Montecucco, Andrea; Siviter, Jonathan; Man, Elena A.; Li, Wen-guang; Paul, Manosh C.; Gao, Min; Sweet, Tracy; Freer, Robert; Azough, Feridoon; Baig, Hasan; Mallick, Tapas K.; Gregory, Duncan H. (2017)
Publisher: Wiley
Languages: English
Types: Article
Subjects: Synthesis, QD, Thermoelectrics, QD Chemistry, Nanomaterials, NDAS, n-type, Tin selenide
This work was financially supported by the EPSRC (EP/K022156/1). SRP and JWGB acknowledge the EPSRC for support (EP/N01717X/1). HFG and WZ acknowledge the EPSRC for the Equipment Grant to purchase Titan Themis 200 microscope (EP/L017008/1). An aqueous solution method is developed for the facile synthesis of Cl-containing SnSe nanoparticles in 10 g quantities per batch. The particle size and Cl concentration of the nanoparticles can be efficiently tuned as a function of reaction duration. Hot pressing produces n-type Cl-doped SnSe nanostructured compacts with thermoelectric power factors optimized via control of Cl dopant concentration. This approach, combining an energy-efficient solution synthesis with hot pressing, provides a simple, rapid, and low-cost route to high performance n-type SnSe thermoelectric materials. Postprint Peer reviewed
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