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Zhao, P.; Lampronti, G.I.; Lloyd, G.O.; Suard, E.; Redfern, S.A.T. (2014)
Publisher: Royal Society of Chemistry
Journal: Journal of Materials Chemistry A
Languages: English
Types: Article
Subjects: sub-03
The crystal structures of zeolitic imidazolate framework 7 (ZIF-7) under various CO2 pressures were studied by high-resolution neutron powder diffraction. CO2 adsorption in ZIF-7 is visualised and demonstrated to be primarily controlled by the benzimidazolate ligands via a gate-opening mechanism. Our results highlight the importance of pressure on the CO2 adsorption and the related structural framework responses in ZIF-7.

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